- Mandy Moore Character (Rapunzel (voice))
- Zachary Levi Character (Flynn Rider (voice))
- Donna Murphy Character (Mother Gothel (voice))
- Ron Perlman Character (Stabbington Brother (voice))
- Jeffrey Tambor Character (Big Nose Thug (voice))
- Brad Garrett Character (Hook Hand Thug (voice))
- Paul F. Tompkins Character (Short Thug (voice))
- Richard Kiel Character (Vlad (voice))
- Delaney Rose Stein Character (Young Rapunzel / Little Girl (voice))
- Nathan Greno Character (Guard 1 / Thug 1 (voice))
- Byron Howard Character (Guard 2 / Thug 2 (voice))
- Tim Mertens Character (Guard 3 (voice))
- Michael Bell Character (Additional Voices (voice))
- Bob Bergen Character (Additional Voices (voice))
- Susanne Blakeslee Character (Additional Voices (voice))
- June Christopher Character (Additional Voices (voice))
- Roy Conli Character (Additional Voices (voice))
- David Cowgill Character (Additional Voices (voice))
- Terri Douglas Character (Additional Voices (voice))
- Chad Einbinder Character (Additional Voices (voice))
- Pat Fraley Character (Additional Voices (voice))
- Eddie Frierson Character (Additional Voices (voice))
- Jackie Gonneau Character (Additional Voices (voice))
- Nicholas Guest Character (Additional Voices (voice))
- Bridget Hoffman Character (Additional Voices (voice))
- Daniel Katz Character (Additional Voices (voice))
- Anne Lockhart Character (Additional Voices (voice))
- Mona Marshall Character (Additional Voices (voice))
- Scott Menville Character (Additional Voices (voice))
- Laraine Newman Character (Additional Voices (voice))
- Paul Pape Character (Additional Voices (voice))
- Lynwood Robinson Character (Additional Voices (voice))
- Fred Tatasciore Character (Additional Voices (voice))
- Hynden Walch Character (Additional Voices (voice))
- Kari Wahlgren Character (Additional Voices (voice))
- M.C. Gainey Character (Captain of the Guard (voice))
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