- Will Ferrell Character (Megamind (voice))
- Brad Pitt Character (Metro Man (voice))
- Tina Fey Character (Roxanne Ritchi (voice))
- Jonah Hill Character (Titan (voice))
- David Cross Character (Minion)
- Justin Long Character (Minions)
- Bill Hader Character (Bob Prickles)
- Amy Poehler Character (Linda Prickles)
- Rob Corddry Character (Random Citizen)
- J.K. Simmons Character (Warden)
- Ben Stiller Character (Bernard)
- Justin Theroux Character (Megaminds's Father)
- Christopher Knights Character (Prison Guard)
- Jack Blessing Character (Newscaster)
- Jessica Benia Character (Megamind's Mother)
- Joey Dinitere Character (Baby Megamind)
- Noah Dinitere Character (Babby Metro Man)
- Lrke Winther Andersen Character (Roxanne (Voice: Danish Version))
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